Theory and Motivation

Isospin symmetry is broken by two-body charge-dependent interactions of the form,

fig1

Such that, for a given nucleus, the total Hamiltonian can be written as the sum of isoscalar, isovector and isotensor operators.  The masses of an isospin multiplet are related by the Isobaric Multiplet Mass equation,

fig2

The IMME is a useful tool to predict level energies and masses of the most exotic members of multiplets when direct measurements are difficult. Checking for deviations from the IMME using measured masses tests the accuracy of such extrapolations.

The A = 32, T = 2 quintet is the most precisely measured quintet so far. We remeasured the mass of the Tz = 0 member of this quintet (32S) with unprecedented accuracy and precision using the 31P(p,γ) reaction. This is a stringent test of the isobaric multiplet mass equation.

Experiment

decaysThe lowest T = 2 state in 32S was produced using the 31P(p,γ) reaction. A proton beam at ≈ 3285 keV was bombarded on an implanted 31P target. The target was seated on a target ladder that allowed for direct water cooling on the Tantalum backing. The corresponding de-excitation γ rays registered using HPGe detectors.  The energies of these γ rays give us the excitation energy of the T = 2 state and thus the mass of the state. The figure on the left shows the gamma decays of the lowest T = 2 state of  32S.

We performed two independent measurements at different times. The first set of data were obtained using two HPGe detectors at +90° and -90° to the beam. These set of gamma-rays had minimal Doppler shift. The energy calibration was done using a 56Co source, and capture radiation from 27Al(p,γ) and 35Cl(n,γ) reactions. Neutrons were produced using the 7Li(p,n) reaction. A proton beam at Ep≈1912 keV impinged a thick Lithium Oxide target (≈ 500 μg/cm2) to produce neutrons that were moderated by a 4 cm thick paraffin slab before capturing on a block of NaCl.

The second set of data were obtained using a HPGe detector at 0° to the beam. The gamma-rays were detected with maximum Doppler shift, but had least sensitivity to target ladder and detector misalignments.  The energy calibration was done using the 56Co source and 27Al(p,γ) lines. The experimental setups are shown below (top view).

zero         ninety calib
Results and Conclusions

spectraSystematic effects such as gain-shifts, Doppler effects and ADC non-linearities were taken into consideration and corrected for to obtain peak centroids. The Doppler effects on γ energies were determined using precise Monte Carlo simulations. Our results agree well with previous determinations of excitation energies of the three T = 1 levels fed by the T = 2 state, but disagree with the previously cited value of the excitation energy of the T = 2 state itself by ≈ 7σ. The figure on the right shows the γ-ray spectrum from the 0° detector.
On using the best available masses for the other members of the T = 2, A = 32 quintet we obtain significant disagreement with the IMME prediction with Q(χ2,ν) = 0.0001. Our result provides the best demonstration of the validity of the approximations inherent in the IMME and its utility for predicting masses away from the valley of stability. The figure below shows the residuals between the IMME fit and measured mass excesses for the quintet.

imme_fit

We investigated the possibility of isospin mixing with other states that would manifest itself in the form of an isospin-violating (ΔT =2) branch. We set an upper limit to this branch (0.25%) and in addition, obtained a new determination of the relative gamma branches from the T = 2 state.  The experimental details and results are explained in greater detail in Phys. Rev. C 73, 054313 (2006).